Detection of nitroaromatic explosives using fluorescent porphyrins entrapped in silica sol-gel matrix

Faculty Mentor(s) Name(s)

Dr. Catrena H. Lisse

Abstract

There is a great need for a reproducible and reusable method for the detection of nitroaromatic explosives and various precursors for many industries, especially homeland security. Fluorescent porphyrin molecules immobilized within silica sol-gels were synthesized and used to study the binding of various nitroaromatics, including 2,4-dinitrophenol, 2,4,6-trinitrophenol, and 1,3-dinitrobenzene. Free-base meso-tetrakis-4-carboxyphenyl porphyrin (H2TCPP) was entrapped within silica sol-gels during the polycondensation process. The interaction of the porphyrin with nitroaromatics, the porphyrin functionality, and the structural integrity of the doped sol-gels were examined using fluorescence and ultraviolet/visible (UV-Vis) spectroscopy. The experimental methodology and preliminary results of the study will be presented.

Start Date

27-3-2024 10:00 AM

End Date

27-3-2024 10:50 AM

Location

Magnolia Ballroom

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Mar 27th, 10:00 AM Mar 27th, 10:50 AM

Detection of nitroaromatic explosives using fluorescent porphyrins entrapped in silica sol-gel matrix

Magnolia Ballroom

There is a great need for a reproducible and reusable method for the detection of nitroaromatic explosives and various precursors for many industries, especially homeland security. Fluorescent porphyrin molecules immobilized within silica sol-gels were synthesized and used to study the binding of various nitroaromatics, including 2,4-dinitrophenol, 2,4,6-trinitrophenol, and 1,3-dinitrobenzene. Free-base meso-tetrakis-4-carboxyphenyl porphyrin (H2TCPP) was entrapped within silica sol-gels during the polycondensation process. The interaction of the porphyrin with nitroaromatics, the porphyrin functionality, and the structural integrity of the doped sol-gels were examined using fluorescence and ultraviolet/visible (UV-Vis) spectroscopy. The experimental methodology and preliminary results of the study will be presented.